Data Underpinning: Magnetic phase diagram of rouaite, Cu₂⁢(OH)₃⁢NO₃

Documentation of the data
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Each experimental technique has its own subdirectory, and each subdirectory has a notes.txt file describing the files therein. In several cases the data are sorted in subdirectories, e.g. by magnetic field direction.

References to related material
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Phys. Rev. B 110, 054442 doi:10.1103/PhysRevB.110.054442

Description of the data
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Data underpinning "Magnetic phase diagram of rouaite, Cu₂⁢(OH)₃⁢NO₃", published as Phys. Rev. B 110, 054442 (2024), doi:10.1103/PhysRevB.110.054442 also available as arXiv:2405.18961 doi:10.48550/arXiv.2405.18961 Contains or describes data from: -specific heat -dilatometry -inelastic neutron scattering -magnetization -AC susceptometry -neutron Laue diffraction -optical microscopy -nuclear magnetic resonance spectroscopy -neutron powder diffraction -thermal transport -ultrasound attenuation

Type of the data
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Dataset

Total size of the dataset
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414232651

Author
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Peets, Darren Campbell

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Mannathanath Chakkingal, Aswathi

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Kulbakov, Anton A.

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Grumbach, Justus

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Pavlovskii, Nikolai S.

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Stockert, Ulrike

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Parui, Kaushick Krishnakanta

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Avdeev, Maxim

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Kumar, Ramender

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Niwata, Issei

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Häußler, Ellen

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Gumeniuk, Roman

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Stewart, J. Ross

Author
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Tellam, James P.

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Pomjakushin, Vladimir

Author
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Granovsky, Sergey

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Doerr, Mathias

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Hassinger, Elena

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Zherlitsyn, Sergei

Author
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Ihara, Yoshihiko

Author
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Inosov, Dmytro S.

Upload date
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2024-11-04T14:36:21Z

Publication date
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2024-11-04T14:36:21Z

Data of data creation
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2024

Publication date
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2024-11-04

Abstract of the dataset
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This contains the data underpinning our recent paper on rouaite, Cu₂⁢(OH)₃⁢NO₃, published in Phys. Rev. B 110, 054442 (2024). The abstract of the article is reproduced below: Spinon-magnon mixing was recently reported in botallackite Cu2⁢(OH)3⁢Br with a uniaxially compressed triangular lattice of Cu2+ quantum spins [H. Zhang et al., Phys. Rev. Lett. 125, 037204 (2020)]. Its nitrate counterpart rouaite, Cu2⁢(OH)3⁢NO3, has a highly analogous structure and might be expected to exhibit similar physics. To lay a foundation for research on this material, we clarify rouaite's magnetic phase diagram and identify both low-field phases. The low-temperature magnetic state consists of alternating ferromagnetic and antiferromagnetic chains, as in botallackite, but with additional canting, leading to net moments on all chains which rotate from one chain to another to form a 90∘ cycloidal pattern. The higher-temperature phase is a helical modulation of this order, wherein the spins rotate from one Cu plane to the next. This extends to zero temperature for fields perpendicular to the chains, leading to a set of low-temperature field-induced phase transitions. Rouaite may offer another platform for spinon-magnon mixing, while our results suggest a delicate balance of interactions and high tunability of the magnetism.

Public reference to this page
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https://opara.zih.tu-dresden.de/handle/123456789/1046

Public reference to this page
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https://doi.org/10.25532/OPARA-659

Publisher
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Technische Universität Dresden

Licence
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Attribution 4.0 Internationalen

URI of the licence text
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http://creativecommons.org/licenses/by/4.0/

Specification of the discipline(s)
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3::32::307::307-01

Specification of the discipline(s)
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3::31::322::322-01

Title of the dataset
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Data Underpinning: Magnetic phase diagram of rouaite, Cu₂⁢(OH)₃⁢NO₃

Underlying research object
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Synthetic rouaite single crystals and powders

Public project website(s)
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https://www.ctqmat.de

Public project website(s)
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https://fis.tu-dresden.de/portal/en/organisations/clusters-of-excellence-ctqmat-complexity-and-topology-in-quantum-matter(7bac147f-30fb-409f-ada3-5381707258b2).html

Public project website(s)
opara.project.publicReference

https://tu-dresden.de/mn/physik/sfb1143

Project title
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Cluster of Excellence 2147, ct.qmat–Complexity and Topology in Quantum Matter; Correlated Magnetism: From Frustration to Topology (SFB 1143); Frustrated Magnetism in Copper Minerals (PE 3318/2-1, PE 3318/2-2)
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This compressed file contains the data files, structured in directories by technique. Each directory contains a notes.txt file with additional information that may be useful for understanding the data files or reproducing our analysis.
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